期刊
ORGANIC LETTERS
卷 19, 期 9, 页码 2358-2361出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00894
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-
资金
- NSFC [21172034, 21372039, 21372038, 21522202]
An ambient-light-promoted and,metal-free three-component reaction of active methylene compounds perfluoroalkyl iodides, and guanidines/amidines is reported: This constitutes a powerful method to prepare prfluoroalky-lated pyrinudines with mild reaction Conditions, broad substrate scope, excellent functional group tolerance, and simple operation. A radical/polar mechanism involving the formation of a halogen-bond adduct and radical cross-coupling is proposed.
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