期刊
ORGANIC LETTERS
卷 19, 期 19, 页码 5328-5331出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b02618
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资金
- Deutsche Forschungsgemeinschaft (DFG) [WU 317/20-1]
Two new bowl-shaped polycyclic aromatic hydrocarbons, based on corannulene and naphthalene dicarboximide, are synthesized by an improved Suzuki-Miyaura cross-coupling and C-H arylation cascade reaction. Crystallographic analyses confirm structural assignments and provide insight into molecular interactions in the solid state. The new bowl-shaped molecules show reversible oxidation and reduction, intense visible range absorption, and high fluorescence quantum yields. These molecules can be considered bowl-shaped congeners of planar perylene dicarboximides.
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