期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 15, 期 2, 页码 324-327出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ob02330d
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资金
- National Natural Science Foundation of China [21502234, 21602256]
- Natural Science Foundation of Shandong Province [ZR2015BL006]
- CAMS Innovation Fund for Medical Sciences (CIFMS) [2016-I2M-3-009]
- Fundamental Research Funds for CAMS/PUMC [2016RC350004]
A silver-catalyzed regioselective C2-alkylation of heteroarenes with tertiary cycloalkanols under radical conditions was developed. This tandem process, which includes selective C-H activation, C(sp(3))-C(sp(3)) bond cleavage, and C(sp(3))-C(sp(2)) bond formation, affords a novel and environmentally friendly approach for the production of carbonyl-containing alkyl-substituted heteroarenes with moderate to good yields.
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