期刊
ACS APPLIED ENERGY MATERIALS
卷 1, 期 11, 页码 5907-5918出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsaem.8b00552
关键词
reduced graphene oxide; ascorbic acid; lemon; paramagnetism; photocatalytic hydrogen production; water splitting
资金
- Department of Science and Technology (SERB), India [SB/S1/PC-31/2012]
- UGC-DAE-CSR Indore [CSR-IC-MSRSR-25/CRS-233/2017-18/1314]
- Ministry of Science and Technology of Taiwan [MOST 107-2113-M-002-008-MY3]
Here, we present the reduction of the graphene oxide (GO) sheets by means of the two reducing agents, i.e., ascorbic acid and lemon juice. As-prepared carbonaceous substances (rGO-AA and rGO-Lemon) exhibits good room temperature (RT) ferromagnetism even in absence of d- and f-electrons as well as they show good hydrogen generation capacity via photocatalytic water splitting. The amount of H2 evolved for Pt/GO, Pt/rGO-AA, and Pt/rGO-Lemon systems was 32.0790, 23.1649, and 38.0790 mmol h(-1) g(-1), respectively. The results go hand in hand and are supported by the reasonably good spin concentration due to the presence of a large amount of the free-radical-like carbon, long-range direct/indirect exchange or interaction between graphene matrix, fragmented graphitic zones, C-defect nonbonding localized electronic states, and flat-band quasi-localized (QL) states induced by the point defects.
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