期刊
NANOTECHNOLOGY
卷 29, 期 2, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/1361-6528/aa9bfe
关键词
1T phase WS2 nanosheets; hydrothermal method; phase stability; TE properties
资金
- National Natural Science Foundation of China [51602306, 61601434]
- Venture & Innovation Support Program for Chongqing Overseas Returnees
- Ministry of Science & ICT (MSIT), Republic of Korea [IBS-R011-D1-2018-A00] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Two-dimensional materials have gained great attention as a promising thermoelectric (TE) material due to their unique density of state with confined electrons and holes. Here, we synthesized 1T phase tungsten disulfide (WS2) nanosheets with high TE performance via the hydrothermal method. Flexible WS2 nanosheets restacked thin films were fabricated by employing the vacuum filtration technique. The measured electrical conductivity was 45 S cm(-1) with a Seebeck coefficient of + 30 mu V K-1 at room temperature, indicating a p-type characteristic. Furthermore, the TE performance could be further improved by thermal annealing treatment. It was found the electrical conductivity could be enhanced 2.7 times without sacrificing the Seebeck coefficient, resulting in the power factor of 9.40 mu W m(-1) K-2. Moreover, such 1T phase WS2 nanosheets possess high phase stability since the TE properties maintained constant at least half one year in the air atmosphere. Notably, other kinds of 1T phase transitional metal dichalcogenides (TMDCs) with excellent TE performance also could be imitated by using the procedure in this work. Finally, we believe a variety of materials based on 1T phase TMDCs nanosheets have great potential as candidate for future TE applications.
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