期刊
NANOSCALE
卷 9, 期 42, 页码 16342-16348出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7nr06374a
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资金
- National Natural Science Foundation of China [U1401248]
- 973 Program - the National Basic Research Program of China Special Funds for the Chief Young Scientist [2015CB358600]
- Excellent Young Scholar Fund from National Natural Science Foundation of China [21422103]
- Suzhou Key Laboratory for Advanced Carbon Materials and Wearable Energy Technologies
- Dongguan Program for International ST Cooperation [2015508102006]
Exploring low-cost and efficient electrocatalysts based on earth-abundant elements for the hydrogen evolution reaction (HER) is of great importance for the development of clean and renewable energy. In this work, we report a facile self-foaming strategy for synthesis of hierarchically interconnected nitrogendoped carbon nanosheets (NCNS). The doping N species within the 3D interconnected carbon network affords rich active sites for the HER and facilitates fast charge transfer. As a result, the NCNS exhibit excellent catalytic activity with an onset potential of -65 mV, and a Tafel slope of 81 mV dec(-1) with robust stability over 10 h in acidic media. Further analyses suggest that the graphitic N species in the NCNS contribute to their catalytic activity. Such a high catalytic performance makes the NCNS a promising metalfree HER electrocatalyst for practical hydrogen production.
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