期刊
NANO LETTERS
卷 17, 期 4, 页码 2634-2639出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.7b00444
关键词
Hexagonal boron nitride; two-dimensional materials; point defects; plasmonic nanocavity arrays; plasmonic coupling
类别
资金
- Australian Research Council [DP140102721, IH150100028, DE130100592]
- FEI Company
- Asian Office of Aerospace Research and Development [FA2386-15-1-4044]
- National Science Foundation (NSF) [DMR-1306514, DMR-1608258]
- State of Illinois
- Northwestern University
- Australian Research Council [IH150100028] Funding Source: Australian Research Council
Quantum emitters in two-dimensional materials are promising candidates for studies of light matter interaction and next generation, integrated on-chip quantum nanophotonics. However, the realization of integrated nanophotonic systems requires the coupling of emitters to optical cavities and resonators. In this work, we demonstrate hybrid systems in which quantum emitters in 2D hexagonal boron nitride (hBN) are deterministically coupled to high quality plasmonic nanocavity arrays. The plasmonic nanoparticle arrays offer a high-quality, low-loss cavity in the same spectral range as the quantum emitters in hBN. The coupled emitters exhibit enhanced emission rates and reduced fluorescence lifetimes, consistent with Purcell enhancement in the weak coupling regime. Our results provide the foundation for a versatile approach for achieving scalable, integrated hybrid systems based on low-loss plasmonic nanoparticle arrays and 2D materials.
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