期刊
ELECTROCHIMICA ACTA
卷 176, 期 -, 页码 207-214出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2015.07.032
关键词
Hydrangea-like; carbon hollow submicron spheres; mesoporous channels; supercapacitor; gravimetric and volumetric capacitance
资金
- NSFC [51402217, 51420105002, 51202165]
- NSFZJ [LY13E020007]
- Zhejiang Science and Technology Project [2014C31155]
Uniform hydrangea-like multi-scale carbon hollow submicron spheres (HCSSg) are fabricated by a simple hydrothermal method using glucose as carbon source and fibrous silicon dioxides spheres as shape guide. Structure characterization suggests that petal-like partially graphitized carbon nanosheets with the thickness of about 10 nm arranged in three dimensions (3D) to form the hydrangea-like hollow spheres (size ranging from 250 to 500 nm) with mesoporous channels, which can be conducive to be a high specific surface area (934 m(2) g(-1)) and bulk density (0.87 cm g(-3)), hierarchical pores structure with good conductivity. As a result, the HCSSg has been demonstrated to be a supercapacitor electrode material with high gravimetric (386 F g(-1) at 0.2 A g(-1)) and outstanding volumetric (335 F cm(-3)) capacitance, good rate capability and cycling stability with 94% capacitance retention after 5000 cycles in aqueous electrolytes, thus suggesting its application potential. (C) 2015 Elsevier Ltd. All rights reserved.
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