期刊
PHYSICAL REVIEW B
卷 99, 期 4, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.99.045308
关键词
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资金
- NSF EFRI [EFMA-1542707]
- NSF CAREER [DMR 1553788]
- AFOSR [FA9550-16-1-0020]
- Cornell Center for Materials Research-an NSF MRSEC [DMR 1719875]
- Leonard Mandel Faculty Fellowship in Quantum Optics
We report on the modulation of the fine-structure splitting of quantum-confined excitons in localized quantum emitters hosted by a monolayer transition metal dichalcogenide (TMDC). The monolayer TMDC, tungsten diselenide (WSe2), is encapsulated in a van der Waals heterostructure which enables the application of an external electric field on the quantum-dot-like emitters hosted by the monolayer flake. The emitters exhibit quantum-confined Stark effect and a modulation in the fine-structure splitting (FSS) as a function of electric field. A maximum modulation of 1500 mu eV is observed in the FSS from the studied emitters. Finally, we measure the polarization response of the localized exciton emission as a function of electric field exhibiting strong circular polarization with decreasing fine-structure splitting, further confirming the suppression of the anisotropic electron-hole exchange interaction thats causes the FSS.
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