期刊
CHEMICAL COMMUNICATIONS
卷 55, 期 7, 页码 917-920出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc09328h
关键词
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资金
- MINECO of Spain [CTQ2015-70795-P]
- Sapienza Universita di Roma (Ricerca Scientifica-Anno 2014)
- MINECO of Spain
Substrate-selectivity stemming from recognition is a key feature of enzymes that has been seldom observed in artificial catalysts. Herein, we report a recognition-driven, substrate-selective C-H oxidation that inverts the intrinsic reactivity of the competing C-H bonds. Analysis of this selectivity highlights an unexpectedly high reactivity enhancement imparted by intramolecularity.
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