期刊
CHEMICAL COMMUNICATIONS
卷 55, 期 11, 页码 1607-1610出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc07185c
关键词
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资金
- European Union through the European Research Council [ERC-AdG-2014-671093]
- Spanish government through the Severo Ochoa Program [SEV-2016-0683]
- Spanish Ministry of Economy and Competitiveness (MINECO) [MAT2016-79776-P]
In this work, we will report the generation of Au clusters in a purely siliceous MCM-22 zeolite. The catalytic properties of these Au clusters have been tested for the selective oxidation of cyclohexane to cyclohexanol and cyclohexanone (KA-oil). The Au clusters encapsulated in the MCM-22 zeolite are highly active and selective for the oxidation of cyclohexane to KA-oil, which is superior to Au nanoparticles on the same support. These results suggest that Au clusters are highly active for the activation of oxygen to produce radical species.
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