期刊
CHEMICAL SCIENCE
卷 10, 期 6, 页码 1780-1785出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8sc04279a
关键词
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资金
- 1000-Youth Talents Plan starting up funding
- National Natural Science Foundation of China [21772183]
- Fundamental Research Funds for the Central Universities [WK2060190086]
- University of Science and Technology of China
In this protocol Ni-catalysed reductive arylalkylation of unactivated alkenes tethered to aryl bromides with primary alkyl bromides has been accomplished, providing a new path to construct diverse benzene-fused carbo- and heterocyclic cores including indanes, tetrahydroisoquinolines, indolines and isochromanes. Notably, this new method circumvents the pregeneration of organometallics and demonstrates high tolerance to a wide range of functional groups. The preliminary mechanistic investigations suggest a reaction pathway with an intermediate reduction.
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