期刊
MICROCHEMICAL JOURNAL
卷 135, 期 -, 页码 91-99出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.microc.2017.08.009
关键词
Covalent triazine frameworks; Peroxidase mimetics; Oxidase mimetics; Biothiol detection
资金
- Sichuan Bureau of Science and Technology [2013kjt003]
A triazine-based covalent organic framework, CTF-1, for the first time, was found to possess both intrinsic peroxidase-like activity and oxidase-like activity and be capable to catalyze the oxidation of chromogenic substrates with or without H2O2 with high efficiency as a robust catalyst. Related oxidization mechanism was thoroughly studied, and the according catalytic properties of CTF-1 was also evaluated. What's more, a facile and effective colorimetric assay was established to detect biothiols without using any oxidizing agents. Compared to natural enzymes and other reported artificial enzymes, CTF-1 has also demonstrated the advantages including low cost, easy preparation, good stability, and high catalytic activity, which made it a very promising enzyme mimetic alternative in potential applications in biosensors for the future. (C) 2017 Elsevier B.V. All rights reserved.
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