4.6 Article

Multicomponent dipolar cycloadditions: efficient synthesis of polycyclic fused pyrrolizidines via azomethine ylides

期刊

ORGANIC & BIOMOLECULAR CHEMISTRY
卷 17, 期 7, 页码 1773-1777

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ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ob02463d

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资金

  1. National Research Foundation of Korea (NRF) [NRF-2016R1A2B4015351, NRF-2016R1A4A1011451]
  2. Government of Korea
  3. Kyung Hee University [KHU-20181169]

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An efficient multicomponent dipolar cycloaddition for the synthesis of polycyclic fused pyrrolizidines was developed using N-aromatic zwitterions, aldehydes, and amino acids. The developed reactions proceed through azomethine ylides generated in situ from the decarboxylated reactions of aldehydes and amino acids followed by the [3 + 2] cycloaddition of N-aromatic zwitterions under mild reaction conditions.

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