期刊
REACTION CHEMISTRY & ENGINEERING
卷 4, 期 3, 页码 550-558出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8re00212f
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资金
- French National Agency [ANR-13-CDII-0001-COUPOX]
- Agence Nationale de la Recherche (ANR) [ANR-13-CDII-0001] Funding Source: Agence Nationale de la Recherche (ANR)
The continuous selective aerobic oxidation of benzyl alcohol in flow was developed using an immobilized Ru-0 catalyst. After optimization of the reaction conditions, the stability and productivity of the equipment were examined over time using tert-amyl alcohol as solvent, and no deactivation occurred. A cumulative TON close to 15000 was obtained with a constant activity (TOF = 4 min(-1)). A semi-empirical kinetic rate expression was proposed.
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