期刊
NEW JOURNAL OF CHEMISTRY
卷 43, 期 8, 页码 3493-3499出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8nj05205k
关键词
-
The electro-reduction of CO2 to produce energy sources has been considered as a visionary pathway with the help of renewable electricity, which can achieve carbon neutrality and mitigate global warming. Nevertheless, developing a high selectivity, good activity and superior stability catalyst is a big challenge. Here, Bi2O3-CuO(x) bimetallic oxide catalysts were synthesized by a facile coordination-precipitation method with concisely controlled atomic ratios (Cu/Bi). They exhibit a remarkable performance for sufficient reduction of CO2 to formate, achieving a maximum faradaic efficiency of 89.3% at a potential of -1.4 V vs. SCE. The catalysts are shown to be robust during 10 h of uninterrupted electrolysis. The notable catalytic activity suggests that controlling the Cu/Bi molar ratio is a key factor in developing special micro-structure Bi2O3-CuO(x) catalysts for electrochemical reduction of CO2 to formate in aqueous systems.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据