期刊
NANOPHOTONICS
卷 8, 期 3, 页码 505-512出版社
WALTER DE GRUYTER GMBH
DOI: 10.1515/nanoph-2018-0211
关键词
ordered colloidal nanostructures; plasmonic field guided patterning; polarization stabilizing
资金
- National Natural Science Foundation of China [11874102, 11474048, 11274058]
Nano-patterned colloidal plasmonic meta-surfaces are capable of manipulation of light at the subwavelength scale. However, achieving controllable lithography-free nano-patterning for colloidal metasurfaces still remains a major challenge, limiting their full potential in building advanced plasmonic devices. Here, we demonstrate plasmonic field guided patterning (PFGP) of ordered colloidal metallic nano-patterns using orthogonal laser standing evanescent wave (LSEW) fields. We achieved colloidal silver nano-patterns with a large area of 30 mm(2) in <10 min by using orthogonal LSEW fields with a non-focused ultralow fluence irradiation of 0.25 W cm(-2). The underlying mechanism of the formation of the nano-patterns is the light-induced polarization of the nanoparticles (NPs), which leads to a dipole-dipole interaction for stabilizing the nano-pattern formation, as confirmed by polarization-dependent surface-enhanced Raman spectroscopy. This optical field-directed self-assembly of NPs opens an avenue for designing and fabricating reconfigurable colloidal nano-patterned metasurfaces in large areas.
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