4.7 Article

B2pin2-catalyzed oxidative cleavage of a C?C double bond with molecular oxygen

期刊

ORGANIC CHEMISTRY FRONTIERS
卷 6, 期 6, 页码 841-845

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c8qo01412d

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资金

  1. National Natural Science Foundation of China [21572195, 21702175]
  2. 1000 Youth Talents Plan
  3. Scientific and Technological Innovation Leading Talent Reserve of Xinjiang Uygur Autonomous Region [wr2016cx0145]
  4. Natural Science Foundation of Xinjiang University [BS160219]

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B(2)pin(2)-catalyzed oxidative cleavage of the C?C double bond of an olefin with molecular oxygen as the oxidant and oxygen source has been developed. Various diaryl ketone, diketone, triketone and estrone derivatives were obtained in moderate to excellent yields. The NMP (N-methyl pyrrolidone)-stabilized B-centered radical species was proposed as a possible catalyst.

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