期刊
MATERIALS SCIENCE & ENGINEERING R-REPORTS
卷 121, 期 -, 页码 1-29出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.mser.2017.09.001
关键词
Lithium-sulfur batteries; Polysulfides; Composite electrodes; Electrolyte; Separators; Mesopore structure
This review is focused on the state-of-the-art of lithium-sulfur batteries. The great advantage of these energy storage devices in view of their theoretical specific capacity (2500 Wh kg(-1), 2800 Wh L-1, assuming complete reaction to Li2S) has been the motivation for a huge amount of works. However, these batteries suffer of disadvantages that have restricted their applications such as high electrical resistance, capacity fading, self-discharge, mainly due to the so-called shuttle effect. Strategies have been developed with the recent modifications that have been proposed as a remedy to the shuttle effect, and the insulating nature of the polysulfides. All the elements of the battery are concerned and the solution, as we present herewith, is a combination of modification of the cathode, of the separator, of the electrolyte, including the choice of binder, even though few binder-free architectures have now been proposed. (C) 2017 Elsevier B.V. All rights reserved.
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