期刊
MATERIALS SCIENCE AND ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS
卷 70, 期 -, 页码 296-302出版社
ELSEVIER
DOI: 10.1016/j.msec.2016.08.077
关键词
Biobased materials; Nanoday; Thermoplastic starch; Poly (butylene adipate-co-terephthalate); Dynamic-mechanical properties
资金
- CAPES [PDSE-9143-12-2]
- CNPq
- Fundacao Araucaria
The effects of sepiolite addition (0, 1, 3 and 5 wt%) were evaluated on dynamic-mechanical behaviour, water uptake, thermal and optical properties of thermoplastic starch (TPS)/poly (butylene adipate-co-terephthalate) (PBAT) nano-biocomposites, with different TPS/PBAT (w/w) ratios and nanofiller contents. The results highlighted the improvement of the dynamic-mechanical behaviour with the addition of sepiolite, producing high performance materials. An increase of 25 degrees C in the T-g of TPS was recorded by DMTA analysis at sepiolite content of 5 wt%. The sepiolite influenced the crystallisation of nano-biocomposites, without causing interference in the crystal organisation, evidenced by DSC analysis. The addition of sepiolite nanoclay decreased the water adsorption rate and water adsorption capacity of the corresponding nano-biocomposites. For such multiphase systems, the successful use of natural sepiolite brought a clear benefit, without the need of any modifications or additional processes to produce advanced nano-biocomposites. (C) 2016 Elsevier B.V. All rights reserved.
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