期刊
MATERIALS RESEARCH BULLETIN
卷 95, 期 -, 页码 607-615出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.materresbull.2017.06.003
关键词
ZnFe2O4/Ag/Ag3VO4; Photocatalytic; Methyl orange; Tetracycline
资金
- National Natural Science Foundation of China for Youths [21407065]
- Natural Science Foundation of Jiangsu Province for Youths [BK20140533]
- China Postdoctoral Science Foundation [2015T80514]
- Priority Academic Program Development of Jiangsu Higher Education
- Jiangsu University Scientific Research Funding [14JDG052]
A novel visible-light driven ZnFe2O4/AglAg(3)VO(4) photocatalyst was successfully fabricated through a two-step hydrothermal method. The structure, morphology arid composition of the samples were characterized by X-ray diffraction (XRD), scanning electron microscope (SEM) and X-ray photo-electron spectroscopy (XPS). The as-prepared ZnFe2O4/Ag/Ag3VO4 composites possessed an excellent performance in the photocatalytic degradation of methyl orange and tetracycline under visible-light irradiation. The results of electrochemical impedance spectroscopy (EIS) indicated that the ZnFe2O4/Ag/Ag3VO4 composite could facilitate the separation of photo-generated carriers, as well as accelerated charge transfer. The 5% ZnFe2O4/Ag/Ag3VO4 composite exhibited the upmost photocatalytic activity, the degradation constant of 5% ZnFe2O4/Ag/Ag3VO4 is as high as 1.49 times to that of Ag/Ag3VO4. Also, according to the trapping experiments, it's found that the superoxide radicals (.O-2) and hole (if) were the predominant reactive species in this system. The ZnFe2O4/Ag/Ag3VO4 photocatalyst is promising for designing as an environmental purification material in treatment of antibiotic pollutant. (C) 2017 Elsevier Ltd. All rights reserved.
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