期刊
NEW JOURNAL OF CHEMISTRY
卷 43, 期 16, 页码 6380-6387出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9nj00176j
关键词
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资金
- National Natural Science Foundation of China [20963009, 21163017, 21563027, 21773187]
In this study, uniform nitrogen-doped hollow carbon spheres (NHCSs) have been synthesized using sphere-like SiO2 as a template and polydopamine as a carbon source. It is found that NHCSs have an ultrahigh specific surface area of 870.1 m(2) g(-1) and high porosity. 9,10-Phenanthrenequinone (PQ) molecules are selected to decorate NHCSs to obtain electrode materials (NHCSs/PQ) for supercapacitors, which show a clear capacitance increase in comparison with pure NHCSs when tested in 1 M H2SO4 aqueous solution. In a three-electrode system, the NHCSs/PQ (mass ratio 4:2) electrodes exhibit larger specific capacitance (as high as 252 F g(-1) at 1 A g(-1)) and an ultrahigh rate capability (80.8% capacitance retention at 30 A g(-1)). Furthermore, the asymmetric supercapacitor is assembled using NHCSs/PQ as a positive electrode material and nitrogen-doped porous carbon (NPCs) that has adsorbed anthraquinone as a negative electrode material, respectively. The device exhibits a high energy density of 8.34 W h kg(-1) along with a power density of 600 W kg(-1).
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