期刊
NPJ 2D MATERIALS AND APPLICATIONS
卷 3, 期 -, 页码 -出版社
NATURE RESEARCH
DOI: 10.1038/s41699-019-0097-3
关键词
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资金
- Indian Space Research Organization (ISRO)
- Nano Mission from the Department of Science and Technology (DST)
- MHRD, MeitY,
- DST Nano Mission through NNetRA
- SERB, DST through NPDF
The possibility of electrical manipulation and detection of a charged exciton (trion) before its radiative recombination makes it promising for excitonic devices. Using a few-layer graphene/monolayer WS2/monolayer graphene vertical heterojunction, we report interlayer charge transport from top few-layer graphene to bottom monolayer graphene, mediated by a coherently formed trion state. This is achieved by using a resonant excitation and varying the sample temperature; the resulting change in the WS2 bandgap allows us to scan the excitation around the exciton-trion spectral overlap with high spectral resolution. By correlating the vertical photocurrent and in situ photoluminescence features at the heterojunction as a function of the spectral position of the excitation, we show that (1) trions are anomalously stable at the junction even up to 463 K due to enhanced doping, and (2) the photocurrent results from the ultrafast formation of a trion through exciton-trion coherent coupling, followed by its fast interlayer transport. The demonstration of coherent formation, high stabilization, vertical transportation, and electrical detection of trions marks a step toward room-temperature trionics.
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