期刊
JOURNAL OF THE ELECTROCHEMICAL SOCIETY
卷 166, 期 10, 页码 H473-H479出版社
ELECTROCHEMICAL SOC INC
DOI: 10.1149/2.1201910jes
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资金
- Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [2018R1D1A3B05042787]
- Human Resources Program in Energy Technology of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Ministry of Trade, Industry & Energy, Republic of Korea [20174030201760]
- Korea Institute of Energy Technology Evaluation and Planning (KETEP)
- Ministry of Trade, Industry & Energy(MOTIE) of the Republic of Korea [20163010012310]
- Korea Evaluation Institute of Industrial Technology (KEIT) [20174030201760] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [2018R1D1A3B05042787] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Cobalt selenide (CoSe2) thin films are successfully formed on F-doped SnO2 (FTO) via a single step potentiodynamic electrodeposition process without any post treatment, and are utilized as counter electrodes (CEs) for dye-sensitized solar cells (DSSCs). The electrochemical behavior of the electrodeposited FTO/CoSe2 films is examined through Tafel polarization, cyclic voltammetry, and electrochemical impedance spectroscopy measurements. The results indicate that the FTO/CoSe2 films exhibit outstanding electrocatalytic ability and electrochemical stability toward the I-/I-3(-) redox couple. The optimized FTO/CoSe2 film fully covers the FTO substrate and features a nanoporous structure of interconnecting nanocrystalline networks, which is beneficial for the diffusion of ions and provides numerous electrochemical active sites. The optimized DSSC using FTO/CoSe2 as CE exhibits a significantly improved cell efficiency of 7.95% compared to that of the DSSC using FTO/Pt as CE (7.48%). (c) 2019 The Electrochemical Society.
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