4.7 Article

Manganese-catalyzed direct C-C coupling of -C-H bonds of amides and esters with alcohols via hydrogen autotransfer

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DALTON TRANSACTIONS
卷 48, 期 21, 页码 7094-7099

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ROYAL SOC CHEMISTRY
DOI: 10.1039/c8dt05020a

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资金

  1. SERB, India [CRG/2018/002480]
  2. Reliance Industries Limited, Navi Mumbai, India
  3. CSIR-SRF
  4. CSIR-NCL
  5. IISER Tirupati

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Herein we report an efficient manganese-catalyzed C-alkylation of unactivated amides and tert-butyl acetate using alcohols as alkylating agents. This elegant approach exhibits a broad substrate scope providing the C-C coupled products of amides via a hydrogen auto-transfer strategy using aryl, heteroaryl, and aliphatic alcohols.

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