4.4 Article

Ultrafast dynamics of electron-phonon coupling in a metal

期刊

EPL
卷 126, 期 5, 页码 -

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IOP PUBLISHING LTD
DOI: 10.1209/0295-5075/126/57001

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资金

  1. Berkeley Lab's program on Ultrafast Materials Sciences - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]
  2. National Research Foundation of Korea (NRF) - Korea government (MSIT) [2017K1A3A7A09016384, 2018R1A2B6004538]
  3. National Research Foundation of Korea [2018R1A2B6004538, 2017K1A3A7A09016384] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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In the past decade, the advent of time-resolved spectroscopic tools has provided a new ground to explore fundamental interactions in solids and to disentangle degrees of freedom whose coupling leads to broad structures in the frequency domain. Time- and angle-resolved photoemission spectroscopy (tr-ARPES) has been utilized to directly study the relaxation dynamics of a metal in the presence of electron-phonon coupling. The effect of photo-excitations on the real and imaginary part of the self-energy as well as the time scale associated with different recombination processes are discussed. In contrast with a theoretical model, the phonon energy does not set a clear scale governing quasiparticle dynamics, which is also different from the results observed in a superconducting material. These results point to the need for a more complete theoretical framework to understand electron-phonon interaction in a photo-excited state. Copyright (C) EPLA, 2019

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