期刊
JOURNAL OF MATERIALS CHEMISTRY C
卷 7, 期 20, 页码 6152-6160出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9tc00483a
关键词
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资金
- National Basic Research Program of China (973 Program) [2009CB939705]
- Platform of Science and Technology and Talent Team Plan of Guizhou province [2017-5610]
- National Nature Science Foundation of China [1174227, 11364005, 11474151, 11774156, 11604060]
- National Science Foundation of Guizhou province [2014-2059]
- Chinese Universities Scientific Fund
The development of efficient strategies for the micro-structural design of microwave absorbers with a thin layer thickness, broad bandwidth, and strong absorption intensity remains a great challenge. In this study, hydrogenated black TiO2 (B-TiO2) nanoparticles (NPs) wrapped by an amorphous carbon (B-TiO2/C) composite were successfully synthesized via a one-step hydrogenation-carbonization method for the first time. The structures and performances of the B-TiO2/C composites could be adjusted by simply altering the carbonization time. The complex permittivity performances of B-TiO2/C under different carbonization times were investigated to optimize its composite structure, which could distinctly enhance its electromagnetic (EM) wave absorption property. The minimum reflection loss (RL) value of -73.2 dB in the roe-like B-TiO2/C was obtained and the effective absorption bandwidth was measured to be 6.8 GHz with a thin thickness of 1.5 mm. The superior microwave absorbing property of the composites originates from the improvement of the impedance matching with the coating of amorphous carbon, which increased the multiple relaxation processes.
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