期刊
ORGANIC CHEMISTRY FRONTIERS
卷 6, 期 13, 页码 2240-2244出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9qo00421a
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资金
- Science&Technology Development Fund of Tianjin Education Commission for Higher Education [2018KJ159]
- Doctoral Program Foundation of Tianjin Normal University [043135202-XB1703]
- National Natural Science Foundation of China [21572160]
- Foundation of Development Program of Future Expert in Tianjin Normal University [WLQR201706, WLQR201811]
- Program for Innovative Research Team in University of Tianjin [TD13-5074]
An efficient approach for the cascade radical cyclization/functionalization of gamma,delta-unsaturated oxime esters was developed, which introduced useful functional groups (-SO2R, -CN, -SCN) into pyrrolines. Control experiments were conducted and a mechanism involving iminyl radical intermediates, which was initiated by Cu(i) species, was proposed.
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