期刊
CHEMICAL COMMUNICATIONS
卷 55, 期 54, 页码 7840-7843出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc03939b
关键词
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资金
- National Natural Science Foundation of China [21871183, 21631007, 21225103]
- Doctoral Fund of Ministry of Education of China [20130002110042]
- Tsinghua University Initiative Foundation Research Program [20131089204]
- State Key Laboratory of Natural and Biomimetic Drugs [K20160202]
- Shanghai Institute of Technology
An efficient oxidation and functionalization of C-H bonds with an inorganic-ligand supported iron catalyst and hydrogen peroxide to prepare the corresponding ketones was achieved using the bromide ion as a promoter. Preliminary mechanistic investigations indicated that the bromide ion can bind to FeMo6 to form a supramolecular species (FeMo6 center dot 2Br), which can effectively catalyze the reaction.
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