期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 139, 期 4, 页码 1388-1391出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b11234
关键词
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资金
- National Natural Science Foundation of China [21402134]
- Natural Science Foundation of Jiangsu Province [BK20140306]
- Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Soochow University
Herein we report a novel, general protocol for distal heteroaryl ipso-migration and its application to the elusive heteroarylation of unactivated alkenes. A set of nitrogen-containing hetero aryl groups showcase the migratory aptitude. This reaction provides a variety of fluoroalkyl functionalized heteroarenes under mild reaction conditions. This is the first report of a difunctionalization of unactivated alkenes with distal heteroaryl migration.
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