期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 139, 期 28, 页码 9459-9462出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b04659
关键词
-
资金
- NSFC/China [21625202, 21672070, 91427304]
It is quite challenging to investigate the dynamics of coordination-driven self-assembly due to the existence of multiple intermediates and many possible processes. By taking advantage of the high sensitivity and efficiency of fluorescence-resonance energy transfer (FRET), FRET was successfully employed to real-time monitor the dynamic behavior of coordination-driven self-assembly. The Forster energy transfer efficiencies and kinetic aspects of a series of discrete, well-defined metallacycles have been determined. Moreover, the dynamic characteristics of these supramolecular assemblies, such as the dynamic ligand exchange, anion-induced disassembly and reassembly, and stability in different solvents, have been investigated by using FRET.
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