期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 139, 期 43, 页码 15304-15307出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b09161
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资金
- GSK-EDB [R-143-000-564-592]
- Ministry of Education of Singapore [R-143-000-613-112]
The first enantioselective formal [5+4] cycloaddition is realized under palladium catalysis to deliver benzofuran-fused nine-membered rings. These medium-sized heterocycles and derivatives undergo unique rearrangements induced by transannular bond formation, resulting in the production of two classes of densely substituted polycyclic heterocycles in excellent efficiency and stereoselectivity.
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