期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 139, 期 10, 页码 3643-3646出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b01096
关键词
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资金
- Singapore National Research Foundation (NRF Fellowship) [R-143-000-477-281]
- Ministry of Education (MOE) of Singapore [R-143-000-613-112]
The first catalytic enantioselective isomerization of secondary allylic alcohols to access ketones with a alpha-tertiary stereocenter is presented. The racemic allylic alcohol substrates can be converted to the enantioenriched ketone products in a stereoconvergent fashion. The use of commercially available catalysts and mild reaction conditions makes this an attractive method in stereo selective synthesis.
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