4.6 Article

Enhanced long wavelength omnidirectional photoresponses in photonic-structured perovskite photodetectors

期刊

JOURNAL OF MATERIALS CHEMISTRY C
卷 7, 期 31, 页码 9573-9580

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c9tc02149c

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资金

  1. Research Grants Council, University Grants Committee of Hong Kong Special Administrative Region, China [GRF/12302817, C5037-18GF]
  2. Hong Kong Baptist University Inter-institutional Collaborative Research Scheme [RC-ICRS/15-16/04]

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Enhanced long wavelength omnidirectional photoresponses in organo-lead triiodide (CH3NH3PbI3) perovskite photodetectors (PDs) have been realized by incorporating a 1-D photonic-structured hole transporting layer (HTL), created by nanoimprint lithography. Our theoretical simulation supports the experimental results, revealing that photonic-structured CH3NH3PbI3 PDs enable efficient light absorption. Photonic-structured perovskite PDs also exhibit faster transient photoresponses as compared to a planar control PD over the wavelength range from UV to NIR. The photoresponsivity of photonic-structured PDs is less dependent on the angle of incident light, arising from the improved light in-coupling over a broader angle range of incident light. In particular, photonic-structured CH3NH3PbI3 PDs with unique features such as polarization-insensitive and enhanced long wavelength omnidirectional photoresponses are very attractive for application in high performance near infrared light detection.

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