期刊
PHYSICAL REVIEW B
卷 100, 期 6, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.100.064515
关键词
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资金
- Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]
- DOE Office of Science [DE-AC02-06CH11357]
- COMPRES under NSF [EAR 11-57758]
- GSECARS through NSF [EAR-1128799]
- DOE [DE-FG02-94ER14466]
- COMPRES, the Consortium for Materials Properties Research in Earth Sciences, under NSF [EAR 1606856]
We present a microscopic study of nematicity and magnetism in FeSe over a wide temperature and pressure range using high-energy x-ray diffraction and time-domain Mossbauer spectroscopy. The low-temperature magnetic hyperfine field increases monotonically up to similar to 6 GPa. The orthorhombic distortion initially decreases under increasing pressure but is stabilized at intermediate pressures by cooperative coupling to the pressure-induced magnetic order. Close to the reported maximum of the superconducting critical temperature at p = 6.8 GPa, the orthorhombic distortion suddenly disappears and a new tetragonal magnetic phase occurs. The pressure and temperature evolution of the structural and magnetic order parameters suggests that they have distinct origins.
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