期刊
CHEMICAL COMMUNICATIONS
卷 55, 期 69, 页码 10281-10284出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc04817k
关键词
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资金
- MICINN [CTQ2015-69568-P, PGC2018-100719-B-I00]
- Fundacion Seneca Region de Murcia [19890/GERM/15]
- Fundacion Seneca
- Ministry of Science, Research and Technology of Iran
We report two ligand-controlled cascade reactions relying on the intramolecular carbopalladation of skipped dienes. The use of a bulky monodentate phosphine ligand affords [4,5]-spirocycles via sequential double carbopalladation, however bidentate phosphines promote a remote beta-C-elimination process which does not rely on the use of strained or sterically hindered substrates.
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