期刊
CHEMICAL SCIENCE
卷 10, 期 34, 页码 7952-7957出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9sc02182e
关键词
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资金
- National Natural Science Foundation of China [21602115]
- 1000-Talent Youth Program [020/BF180181]
- Natural Science Foundation of Tianjin [18JCYBJC20400]
- Fundamental Research Funds for the Central Universities
- Nankai University
Herein, we report three-component vicinal-diarylation of non-conjugated alkenes initiated by transmetalation of arylboronic acids, which provides complementary access to beta,gamma-diaryl carbonyl compounds. We have also screened a large number of chiral ligands for developing an enantioselective version of this reaction and obtained the preliminary results (up to 79 : 21 e.r.). Notably, the methodology developed herein represents the first three component syn-vicinal-dicarbofunctionalization of non-conjugated alkenes involving palladium catalysis.
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