期刊
NANOSCALE
卷 11, 期 32, 页码 15037-15042出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9nr02103e
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资金
- Joint Foundation of Liaoning Province Natural Science Foundation [20180510047]
- Shenyang National Laboratory for Materials Science [20180510047]
- National Natural Science Foundation of China [51872115, 21761132025, 21773269, 51372095, 51521091]
- Youth Innovation Promotion Association from the Chinese Academy of Sciences [2015152]
- Program for the Development of Science and Technology of Jilin Province [20190201309JC]
- Open Project Program of Wuhan National Laboratory for Optoelectronics [2018WNLOKF022]
- Jilin Province/Jilin University co-Construction Project-Funds for New Materials [SXGJSF2017-3, Branch-2/440050316A36]
- Program for JLU Science and Technology Innovative Research Team (JLUSTIRT)
- Double-First Class Discipline for Materials Science Engineering
- Natural Science Foundation of Anhui Province [1608085ME93]
- Fundamental Research Funds for the Central Universities [JZ2018YYPY0305]
Interfacial contacts within electrodes largely affect electronic transport and ion migration. Nanoscale electrode materials can achieve high reactivity, but their large interfacial contact areas lead to unavoidable impedance. Herein, a Ti3C2Tx MXene was used to construct a hybrid three-dimensional electrode material with a bilayer feature via a two-step vacuum filtration process. The introduced MXene flakes contributed to the electrode capacity, increased the electronic/ionic conductivity as a conductor and current collector, and enhanced the mechanical behaviour of the electrode by acting as a substrate. Such bilayer hybrid electrode design achieved promising cycling stability, and unlock an electrode architecture that can be applied to a wide range of two-dimensional materials.
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