期刊
JOURNAL OF RAMAN SPECTROSCOPY
卷 48, 期 12, 页码 1881-1886出版社
WILEY
DOI: 10.1002/jrs.5262
关键词
chirping; coherent anti-Stokes Raman scattering; combustion diagnostics; ultrafast nonlinear optics
类别
资金
- NSF [CHE-1361516]
- W. M. Keck foundation
- Direct For Mathematical & Physical Scien [1361516] Funding Source: National Science Foundation
- Directorate For Engineering [1605533] Funding Source: National Science Foundation
- Division Of Chemistry [1361516] Funding Source: National Science Foundation
- Div Of Chem, Bioeng, Env, & Transp Sys [1605533] Funding Source: National Science Foundation
The influence of probe laser chirp on hybrid femtosecond/picosecond pure-rotational coherent anti-Stokes Raman scattering is studied theoretically and experimentally. Experiments of N-2(hybrid fs/ps pure-rotational coherent anti-Stokes Raman scattering) are carried out using an in-house built second harmonic bandwidth compressor, results with different probe chirps of are reported. The experimental spectra are fitted with and without considering probe chirp. Including the chirp improves the fit to experimental spectra at all probe delays. The effect of probe pulse chirp is evaluated through a quantitative analysis of matching residuals.
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