期刊
CHEMICAL COMMUNICATIONS
卷 55, 期 76, 页码 11366-11369出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc05205d
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资金
- Engineering and Physical Sciences Research Council (EPSRC) Centre for Doctoral Training in Sustainable Chemistry [EP/S022236/1]
- European Union's Horizon 2020 research and innovation programme through a Marie Sklodowska-Curie Individual Fellowship [702386]
- University of Nottingham
- GlaxoSmithKline
- Marie Curie Actions (MSCA) [702386] Funding Source: Marie Curie Actions (MSCA)
The synthesis of functionalized 1-tetralones by the rhodium(i)-catalyzed reaction of alkynyl malonates with arylboronic acids is described. These arylative cyclizations proceed via an alkenyl-to-aryl 1,4-Rh(i) migration as a key step. Preliminary results of an enantioselective variant of these reactions are also presented.
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