期刊
CHEMICAL COMMUNICATIONS
卷 55, 期 74, 页码 11111-11114出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc05695e
关键词
-
资金
- National Natural Science Foundation of China [21625203, 21871126]
- Jiangxi Province Science and Technology Project [20182BCB22007, 20181BAB213002]
A new, general silver-catalyzed oxidative 1,2-alkyletherification of unactivated olefinic ketones with primary, secondary and tertiary alpha-bromoalkyl carbonyls promoted by tert-butyl hydroperoxide (TBHP) and Et3N has been developed. Through the cooperative action of Ag2O, TBHP and Et3N, the reaction enables the construction of highly valuable quaternary-carbon-possessing 2,3-dihydrofuran frameworks using a concomitant intramolecular annulation strategy.
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