期刊
PHYSICAL REVIEW B
卷 100, 期 14, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.100.144413
关键词
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资金
- National Basic Research of China [2016YFA0300701, 2017YFA0206300, 2014CB920902]
- National Natural Science Foundation of China [11520101002, 51590880, 11674378]
- Key Program of the Chinese Academy of Sciences
Based on density functional theory calculations, we show how symmetry mismatch at interface induces perpendicular magnetic anisotropy (PMA) for the perovskite/brownmillerite-typed La1/2Sr1/2MnO3/LaCoO2.5 superlattices in different strain states. We found strong interfacial reconstructions, which result in considerable orbital hybridization due to distortion/tilting of the MnO6 octahedron and CoO4 tetrahedron. We identified the orbital pairs that strongly affect magnetic anisotropy, showing that tuning the degree of orbital hybridization by lattice strain is an effective approach to tune magnetic anisotropy. Remarkably, not only octahedron-coordinated Mn ions but also tetrahedron-coordinated Co ions contribute to PMA. This work presents a guidance for tuning spin orientation by interface engineering.
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