期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 82, 期 14, 页码 7683-7688出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.7b01255
关键词
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资金
- National Natural Science Foundation of China [21602086, 21672028]
- Natural Science Foundation for Colleges and Universities of Jiangsu Province [16KJB150002]
- Jiangsu Key Laboratory of Advanced Catalytic Materials Technology [BM2012110]
A metal-free 1,2-alkylarylation of allylic alcohols with aliphatic aldehydes through concomitant radical neophyl rearrangement was developed, providing 1,2-diphenyl-3-alkyl propanones in moderate to good yields. Moreover, when cyclopropanecarbaldehyde and aryl carbaldehydes were concerned, acylarylation was involved leading to 1,4-dicarbonyl compounds.
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