期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 82, 期 15, 页码 8191-8198出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.7b00804
关键词
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资金
- National Key Research and Development Program of China [2016YFA0602900]
- National Natural Science Foundation of China [21420102003]
- Fundamental Research Funds for the Central Universities [2015ZY001]
The first example of Pd-catalyzed oxidative cyclization of allyltosylamides with acetic acid is reported. This transformation involved C-N/C-C bond formation and provided 3-pyrrolin-2-ones in a one-pot manner with easy-operation, excellent atom economy and good yields. Mechanistic studies indicate that the reaction proceeds through intermolecular aminopalladation, migratory insertion, reinsertion and beta-hydride elimination processes.
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