期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 82, 期 23, 页码 12827-12833出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.7b02193
关键词
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资金
- Russian Science Foundation [17-73-20070]
- Russian Science Foundation [17-73-20070] Funding Source: Russian Science Foundation
Active methylene compounds react with in situ generated nonstabilized azomethine ylides via the domino Mannich reaction-dipolar cycloaddition to form 3,3-disubstituted pyrrolidines, including oxindole alkaloids. When the starting material possesses a single activated hydrogen, the reaction terminates at the Mannich base stage. The developed methodology was applied to a short and efficient synthesis of (+/-)-horsfiline and N-protected (+/-)-coerulescine.
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