期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 21, 期 42, 页码 23620-23625出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cp04427b
关键词
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资金
- National Research Foundation of Korea through the Basic Science Research program [2017R1A2B1010215]
- National Creative Research Initiative Grant [2014R1A3A2030423]
- Ministerio de Economia y Competitividad of Spain [CTQ2015-65033-P, PGC2018-096444-B-I00, FIS2016-77889-R]
- Comunidad de Madrid [Y2018/NMT-5028]
- Severo Ochoa Programme for Centres of Excellence in RD (MINECO) [SEV-2016-0686]
- Maria de Maeztu Programme for Units of Excellence in RD [MDM-2014-0377]
- National Research Foundation of Korea [2017R1A2B1010215] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
We predict anti-alignment dynamics in the excited state of H-2(+) or related homonuclear dimers in the presence of a strong field. This effect is a general indirect outcome of the strong transition dipole and large polarizabilities typically used to control or to induce alignment in the ground state. In the excited state, however, the polarizabilities have the opposite sign compared to those in the ground state, generating a torque that aligns the molecule perpendicular to the field, deeming any laser-control strategy impossible.
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