期刊
JOURNAL OF MODERN OPTICS
卷 64, 期 10-11, 页码 1042-1053出版社
TAYLOR & FRANCIS LTD
DOI: 10.1080/09500340.2016.1278282
关键词
Femtosecond laser pulses; ultrafast pulse shaping; two-colour time-resolved photoelectron spectroscopy; strong-field coherent control; rapid adiabatic passage; selective population of dressed states
类别
资金
- Deutsche Forschungsgemeinschaft via QUTIF [SPP 1840]
- Deutsche Forschungsgemeinschaft
Strong-field coherent control deals with the efficient excitation of a quantum system into a preselected final state. In order to understand the underlying control mechanisms, the transient dynamics of the laser-dressed states need to be considered in addition. In this paper, we present a route towards a complete picture of non-perturbative coherent control. To this end, we study near-resonant chirped excitation of potassium atoms as a model system for resonant strong-field control. Combining a two-colour pump-probe scheme with photoelectron spectroscopy, we simultaneously observe final state and transient excitation dynamics in the strongly driven atom. As demonstrated on the prototype scenario, the scheme enables a detailed understanding of the physical mechanisms governing the interaction. Our results highlight the power of two-colour time-resolved photoelectron spectroscopy to shed light onto the different aspects of non-perturbative coherent control.
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