期刊
JOURNAL OF LUMINESCENCE
卷 188, 期 -, 页码 60-66出版社
ELSEVIER
DOI: 10.1016/j.jlumin.2017.04.010
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类别
资金
- EC FP7, Marie Curie Initial Training Network LUMINET [316906]
- Grant Agency of the Czech Technical University in Prague [SGS16/244/OHK4/3T/14]
- NCBR Era-Net NANOLUX project [286]
- NCBR Ukrainian project [SL-20F]
The luminescence and scintillation properties of gadolinium terbium aluminium garnet single crystalline films, Gd3-xTbxAl5O12, doped with Ce3+ are investigated as a function of the Gd/Tb ratio with the aim of an improved understanding of the energy transfer processes between Ce3+ and Tb3+ ions in the aluminium garnet hosts. Upon replacing the Gd3+ by Tb3+, the crystal field splitting for the 5d energy level of Ce3+ does not change significantly, due to comparable sizes of the Gd3+ and Tb3+ cations. Temperature dependence of the decay time of Tb3+ and Ce3+ luminescence confirms an efficient energy transfer from the Tb3+ to Ce3+ and provides a qualitative understanding of this process. Furthermore, bidirectional energy transfer processes between the Ce3+ and Tb3+ are revealed. Scintillation decays under alpha-particles excitation show the presence of the fast and slow sub-microsecond components.
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