期刊
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
卷 45, 期 -, 页码 296-300出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.jiec.2016.09.037
关键词
Methanol; Dimethoxymethane; Selective oxidation; Vanadium oxide; Oxygen
VOx-based catalysts showed good performance in selective oxidation of methanol to dimethoxymethane (DMM). For VOx/TS-1 catalyst, the experiments of Temperature Programmed Surface Reaction (TPSR), in situ Infrared spectrometer (in situ IR) and X-ray photoelectron spectroscopy (XPS) were carried out to investigate the products distribution of the methanol oxidation reaction and the adsorb-desorption process at active centers. Furthermore, the role of oxygen species during the reaction process over VOx/ TS-1 catalyst and the surface reaction mechanism was explored. (C) 2016 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
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