期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 7, 期 45, 页码 25845-25852出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9ta09598e
关键词
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资金
- Natural Science Foundation of Hebei Province [E2019208308, E2019208179]
- Science Foundation of University of Hebei Province [BJ2019036, ZD2019062]
- Science Research and Development Program of Shijiazhuang [181790411A]
The abundance and low cost of potassium resources make potassium ion batteries (PIBs) a future energy storage system. However, it is difficult for current electrode materials to offer enough space to stably store large-sized potassium ions. In this study, using sycamore leaves as the raw material, a porous carbon microtube (PCM) array derived from carbon quantum dots (CQDs) is obtained. The resulting PCM features a multihole cross profile, high surface area (300.3 m(2) g(-1)), and much larger interlayer spacing (0.396 nm). The experimental results and finite element analysis show that the PCM has a strong stable structure to release the stress against pulverization during cycling. As an anode material for PIBs, the PCM electrode displays a capacity of 177.6 mA h g(-1) over 2000 cycles at a very high current density of 2000 mA g(-1), which is among the best high-rate stabilities ever reported. In terms of cost effectiveness, long cycle lifespan and mass production, this work represents a brilliant prospect of anode materials for PIBs.
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